User:David MacQuigg/Sandbox/Integral Fast Reactor

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The Integral Fast Reactor (IFR) is Argonne Lab's best design, a metal-fueled, sodium-cooled, pool-type Fast Neutron Reactor, addressing all the issues raised in Nuclear_power_reconsidered (safety, waste management, weapons proliferation, and cost). "Integral" refers to the on-site reprocessing of the spent fuel.

Fig.1 Fuel rod with high burnup and inherent safety.

Fig.2 Pool-type reactors have enormous heat capacity, and molten sodium will expand when hot, allowing convection to cool the core if the pump ever fails.

Choice of Fuel and Coolant

The IFR has a unique design for its fuel rods that accommodates much higher burnup than in light water reactors (LWRs) and also provides inherent safety if temperatures increase. To contrast IFR fuel with LWR oxide fuel, LWR fuel is "strong fuel, weak cladding", and IFR fuel is "weak fuel, strong clad".

In standard light water reactor (LWR) fuel rods, the lower thermal conductivity of UO2 results in high fuel temperatures that increase fission gas swelling. To avoid fuel-clad mechanical interaction that can cause cladding failure, the fuel-clad gap is filled with helium gas for thermal bonding. If burnup is too high, however, the swelling and/or the oxide fuel cracking from thermal stresses will cause mechanical contact and strain the cladding to failure. These problems have been addressed in LWR fuel designs, but maximum burnup is limited by these effects.

In metallic IFR fuel, the fuel thermal conductivity is much larger than it is for UO2, so the fuel temperature and consequent fission gas swelling more moderate. Fission gas more readily escapes the fuel meat and accumulates in the plenum above the fuel without unduly increasing the fuel rod internal pressure. As in LWR fuel, a radial gap between fuel and clad is put in fresh fuel, with the gap filled with liquid metal sodium as the thermal bond. Because metal fuel is weaker than UO2, mechanical contact with the clad is less consequential. The IFR fuel rod is described in Figure 1.

In oxide-fueled LWRs clad with zirconium alloy, two chemical effects are disadvantagous. First, as happened at Fukushima, if the cladding temperature becomes too high in the presence of water, the zirconium alloy clad (used because of its low neutron capture cross section) rapidly oxidizes, weakening the cladding and producing elemental hydrogen gas. Second, in the event of a cladding breach, the oxide fuel meat reacts with water and corrodes. In the IFR, parasitic fast neutron capture in cladding is far lower than parasitic thermal neutron capture in LWR cladding so steel cladding is used without adversely impacting the neutron economy. Steel does not suffer the rapid oxidation or hydrogen generation at high temperature that zirconium alloys do. If there is a cladding breach, fission products entering the coolant are bound there rather than released.

The thermal expansion coefficient of metallic fuel provides a negative reactivity feedback. If the fuel temperature increases, the fuel and coolant both expand, increasing neutron leakage from the core and thereby reducing the neutron chain reaction naturally. In other words, the temperature and power reactivity feedback coefficients are negative -- the hallmark of a stable system.

The Fuel Cycle

As in other fission reactors, the spent fuel is a mixture of uranium, transuranics, fission products, and fuel material diluents. In LWRs, recycling fuel material more than one time becomes impractical, but the IFR’s fast neutron spectrum makes repeated recycling entirely feasible. The IFR fuel cycle chemistry, pyroprocessing, is the "Goldilocks" chemistry -- good enough to recycle the materials into the reactor again, but not so selective as to make the recycled material attractive for diversion for a nuclear device. It uses electrochemical deposit of the recycle material on a cathode in a molten salt bath, rather like the re-deposit of lead on the electrode in a lead-acid battery. The chemistry of the IFR fuel recycling process does not allow extraction of pure plutonium, and many of the radioactive rare earth fission products stay in the recycled fuel material. This makes the material unattractive from a nuclear weapons material diversion standpoint -- it is too radioactive, contains non-fissile uranium, and is processed either in a highly radioactive argon-gas-atmosphere hot cell or as fully formed highly radioactive fuel elements. Further chemical separation and probably isotopic enrichment would be required, a situation not different in kind from starting with unprocessed fuel. So the IFR adds little or nothing to proliferation risk. The recycle system demonstrated at Argonne National Laboratory over the decades is a batch process that does not require hundreds or thousands of miles of piping containing concentrate nitric acid bearing radioactive material, so it is expected to be substantially cheaper than the aqueous reprocessing used outside of the United States<reference to Plentiful Energy here>. Recycle facilities could economically service a cluster of IFR reactors co-located at one site, as was the case with EBR-II at Argonne-West. In countries not licensed for fuel processing, return of the spent fuel to a secure location could be handled as any other reactor with solid fuel rods. Rods are easy to count, and the number in transit at any one time can be small enough to avoid theft of a large quantity.

Safety

The safety of the IFR design is ensured by several features:
1) The metal fuel, a low melting point alloy of U-Pu-Zr, will melt if the rod ever gets too hot. The fuel then expands upward in the steel cladding, shutting down the fission reactions (see Figure 1). The IFR is "walk away safe".
2) Many of the fission products bind chemically with sodium, reducing the risk of fission product release if there is fuel failure.
3) Convection and a large thermal inertia in the large pool of molten sodium will easily handle the decay heat after a shut-down (see Figure 2).
fuel 4) The reactor vessel has no penetrations below the top of the pool, eliminating the possibility of sodium leakage.
5) There is no high pressure or any water near the reactor vessel.
6) The entire reactor vessel is not filled solid, to allow for thermal expansion and contraction during operation. The space above the sodium pool is filled with argon gas so that air never contacts the sodium.
Full-scale reactor tests were conducted at Argonne National Laboratory (West) in Idaho (now Idaho National Laboratory), in which the primary coolant pump was stopped with the reactor running at full power. All safety systems were disabled, and the control rods were held fully withdrawn. These "unprotected loss-of-flow tests" simulate the extreme scenario where all safety systems and operator actions have failed. The chain reaction was terminated by core expansion, and the core was cooled by natural circulation, without fuel damage or radioactive leakage.

Waste Management

Fuel rods have an advantage over molten salt fuels in that the fission products are contained in the rod. This means a smaller volume of radioactive spent fuel. Also rods are easy to identify and count, which may be advantageous in preventing diversion. A typical 500 MWe MSR produces 13 tonnes of spent nuclear fuel salt per year. A 500 MWe PWR (they are normally about 1000 MWe) would produce about 11 tonnes of heavy metal and fission product waste per year. A 500 MWe IFR would produce about 5 tonnes per year of heavy metal and fission product waste per year. Note: SNF can be reprocessed, and the final amount of HLW will depend on the details of that process.

Weapons Proliferation

The chemistry of the IFR fuel process does not allow extraction of weapons-grade material at any point in the cycle. Spent fuel is a mix of uranium, plutonium, and various actinides. Processing would be necessary by some other unrelated process, a situation not different in kind from starting with unprocessed fuel. So the IFR adds little or nothing to proliferation risk. In countries not licensed for fuel processing, return of the spent fuel to a secure location could be handled as any other reactor with solid fuel rods. Rods are easy to count, and the number in transit at any one time can be small enough to avoid theft of a large quantity.

Cost

• No enormous pressure vessel with 6-inch steel walls.
• No huge containment building with 6-foot think, steel reinforced concrete walls.